For the detection of 241Am at 60 KeV for example, the pulse shape, electronic dead time, discriminator window, and Compton effect in the sample are very important (14 and 81). The intensities of gamma rays and X-rays in 241Am alpha decay has been reported by Magnusson (57) detected with a 0.3 cm thick NaI(T1) scintillator. Presently more accurate decay schemes are available such as in Lederer et al. (53). A detailed spectrum of 241Am radiation shows many other peaks beyond the main peak energy of 59.6 KeV. The most important of these are the 17.5 and 103 KeV energy peaks. When the spectrum was taken with a NaI(Tl) detector, sometimes a 32 KeV escape peak and a region of summation were observed. Because of these unwanted radiation peaks, the window discriminator for the gamma spectrophotometer must be correctly adjusted. A good rule is to adjust the energy window with the same thickness as the crystal resolution for that ..neig\. A thin window decreases the photon counts due to the scattering provided by the Compton effect in the sample. This is par- ticularly important if the collimator solid angle is large. The Compton effect in the sample is important for low energy pho- tons, i.e. when E/Eo < 1 where E is the incident photon energy, Eo is the electron rest energy moC2, and C is the speed of light. For low energy photons, the Compton effect equation which shows the photon wave length variation as a fraction of the scattering angle, a, may be presented as: AE E (1 cosa). [10] E Eo This equation states that loss of energy is very small for large values of the angle a and the scattered photon energy, E', is approximately the same as the incident photon energy E. The angular distribution of the Compton effect is not isotropic and has been described with the Klein- Nishina equation by Evans (24) and by Heitler (46). Ignoring the small influence of multiple scattering, the contribution due to the Compton effect is less than 0.5% for collimators with solid angles less than 6 on the detector side. Cisler et al. (8) reported the influence of the Compton effect upon the counts and Groenevelt et al, (40) reported the influence of the Compton effect upon mass attenua- tion coefficients measured with IJtlerent collimator geometry. After ex- tending the work of Conner et al. (9), Gopal and Sanjeevaiah (38) con- cluded that the effect of multiple scattering upon determinations of mass attenuation coefficients could be greatly minimized by always maintain- ing the product tkx (mass attenuation coefficient and sample thickness) as less than one mean free path. A finite resolving time in measurements of radiation intensity for the garnma ray spectrometer contributes to a coincidence loss or counting 17